From the aerial parts ofNauclea officinalis (Pierre ex Pitard) Merr. et Churl, one new indole alkaloid paratunamide E (1) has been isolated together with six known indole alkaloids, paratunamide A (2), nauclealotide C (3), nauclealotide A (4), vincosamide (5), strictosamide (6) and naucleamide F (7). Naucleamide F (7) was isolated from Nauclea officinalis for the first time. All of the seven compounds above were elucidated by spectroscopic methods including 1 D and 2 D NMR soectroscoDic analyses.
One new ent-pimarane diterpenoid ent-16-nor-3-oxo-pimar-8(14)-en-15-al (1) together with four known diterpenoids kirenol (2), ent-2-oxo-15,16,19-trihydroxypimar-8(14)-ene (3), darutigenol (4) and darutoside (5) were isolated from the ethanol extract of Siegesbeckia pubescens. The planar structures and relative configurations of these compounds were elucidated by comprehensive spectroscopic analysis.