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国家自然科学基金(405320514)

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Distribution and speciation of mercury in the Hongfeng Reservoir,Guizhou Province, China被引量:5
2008年
The water, pore water, sediment, and fish samples were collected from the Hongfeng Reservoir in No- vember 2003 and February 2004 in accordance with trace metal protocols. The average concentrations of total mer- cury (THg), dissolved mercury (DHg), reactive mercury, dissolved gaseous mercury, total methylmercury, and dis- solved methylmercury in the water columns were 8.00, 5.70, 0.63, 0.05, 0.16, and 0.07 ng/L, respectively. THg and DHg in the water columns, THg in pore water and THg in lake sediments of the Hongfeng Reservoir showed the level of mercury in the Hongfeng Reservoir was higher than in other natural waters in the world due to the loading of a lot of waste water with relatively high concentrations of mercury, whereas methylmercury concentrations in fish (wet weight) varied from 1.73–51.00 ng/g, much lower than in most remote lakes and reservoirs reported in northern Europe and North America. Methylmercury distributions in pore water and sediments showed methylation oc- curred mainly in the upper several centimeters of sediment cores in the Hongfeng Reservoir. The concentrations of dissolved organic carbon, total suspended particles, total Hg, and methylmercury were higher at Houwu than those at Daba in November 2003. It is suggested that other pollutants such as N and P from fishing farm and other waste water at Houwu,which resulted in deterioration of water quality, affected the concentrations and distributions of mercury species in the reservoir.
HE TianrongFENG XinbinGUO YannaQIU GuangleYAN HaiyuMENG Bo
关键词:水银生物环境
长白山地区大气气态总汞含量的季节性特征研究被引量:36
2008年
利用高时间分辨率自动大气测汞仪(Tekran 2537A),于2005-08~2006-07对长白山地区大气气态总汞进行了连续1a的野外观测.结果表明,长白山地区气态总汞的年平均含量为(3.22±1.78)ng·m^-3,按季节表现为:冬季〉春季〉秋季〉夏季.长白山地区气态总汞含量高于北半球大气汞含量的背景值(1.5~2.0 ng·m^-3),表明该地区已受到一定程度的大气汞污染.在对长白山地区气态总汞来源的解析中,该区频率最高的指示风向西南(SW)、西北(NW)和非主导风向东北(NE)方位上,城镇人为采暖、燃煤以及对生物燃料的使用成为该地区的气态总汞的主要来源,而土壤释放或其他来源的大气汞经中长距离的迁移也是造成该区域大气汞含量升高的原因.
万奇冯新斌郑伟Lu Y-Julia韩士杰徐浩
关键词:气态总汞
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