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国家自然科学基金(41171057)

作品数:7 被引量:37H指数:3
相关作者:李忠勤张明军王飞腾王圣杰冯芳更多>>
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发文基金:国家自然科学基金国家重点基础研究发展计划中国科学院知识创新工程重要方向项目更多>>
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Characteristics and source of aerosols at Shiyi Glacier,Qilian Mountains, China
2016年
Aerosol samples were collected in the Shiyi Glacier, Qilian Mountains from July 24 to August 19, 2012 and analyzed for major water-soluble ionic species(F^-, Cl^-, NO_2^-, NO_3^-, SO_4^(2-), Na^+, NH_4^+, K^+, Mg^(2+) and Ca^(2+)) by ion chromatography. SO_4^(2-) and NH_4^+ were the most abundant components of all the anions and cations, with average concentrations of 94.72 and 54.26 neq/m^3, respectively, accounting for 34% and 20% of the total water-soluble ions analyzed. These mean ion concentrations were generally comparable with the background conditions in remote sites of the Qilian Mountains, but were much lower than those in certain cities in China. The particles were grouped into two dominant types according to their morphology and EDX signal: Si-rich particles and Fe-rich particles. Backward air mass trajectory analysis suggested that inland cities may contribute some anthropogenic pollution to this glacier, while the arid and semi-arid regions of central Asia were the primary sources of the mineral particles.
XiaoYu ZhangZhongQin LiPing ZhouShengJie Wang
关键词:AEROSOLGLACIERSCANNING
中国天山冰川积雪中NO_3^-与NH_4^+的分布特征及其环境意义被引量:1
2013年
基于2004-2009年间在天山托木尔峰青冰滩72号冰川、奎屯河哈希勒根51号冰川、乌鲁木齐河源1号冰川、博格达峰四工河4号冰川与庙尔沟平顶冰川积累区采集的雪坑样品,分析了中国天山冰川积雪中NO3-与NH4+的空间分布特征及其环境意义.结果表明,积雪中NO3-平均浓度顺序为哈希勒根51号冰川<乌鲁木齐河源1号冰川<庙尔沟平顶冰川<青冰滩72号冰川<四工河4号冰川,而NH4+平均浓度顺序为青冰滩72号冰川<哈希勒根51号冰川<庙尔沟平顶冰川<乌鲁木齐河源1号冰川<四工河4号冰川.结合HYSPLIT空气轨迹模型与局地环境状况资料分析,这种空间差异受到远源污染与沙漠粉尘传输、近源工农业生产与生活排放、冰川积累区地理环境等因素的综合影响.
王圣杰张明军李忠勤王飞腾张晓宇
关键词:冰川积雪硝酸根
基于大气沉降与径流的乌鲁木齐河源区氮素收支模拟被引量:4
2012年
选取天山乌鲁木齐河源区作为自然状态下内陆河源区的代表,将区域氮循环简化为大气沉降输入与径流输出,模拟了该区域内的氮素收支状况,得出结论:(1)乌鲁木齐河源区(总控制水文点以上区域)的年均氮素干湿沉降量为17.0 t/a,且以有机氮为主,其次为铵态氮与硝态氮;年均氮素沉降通量为5.92 kg·hm-2·a-1,明显小于下游受人类活动影响更为强烈的地区。(2)河源区氮素的径流输出主要包括大气沉降直接随径流流失、冰川融水流失与泥沙输移流失等,在总控制水文点以上区域以泥沙输移为主,其次为大气沉降直接随径流流失,冰川融水携带氮量相对较少。(3)河源区氮素的输入量普遍小于输出量,该区域表现为一个氮源;在仅计算大气沉降与径流的情况下,总控制水文点以上区域的年均氮素净通量为-2.64 kg·hm-2·a-1,若将生物固氮与反硝化作用纳入考虑则氮源效应更加显著。
王圣杰张明军王飞腾李忠勤
关键词:氮循环内陆河冰川区
Recent glacial retreat and its effect on water resources in eastern Xinjiang被引量:23
2011年
The eastern Xinjiang Basin is desperately short of water. Most rivers in the basin originate in the high eastern Tianshan, which has abundant precipitation and numerous alpine glaciers. Fieldwork conducted on three reference glaciers around Mt. Bogda in 1981 and 2009 suggests that they all strongly melt in summer, a process that has tended to accelerate in recent decades. Based on topographic maps from 1962 and 1972 and 2005/2006 satellite imagery, we investigated 203 glaciers near Mt. Bogda and 75 glaciers near Mt. Harlik. The results show that the surface area of the Mt. Bogda glaciers decreased by 21.6% (0.49% a?1) from 1962 to 2006. This was accompanied by a 181 m decrease in length and a 28% drop in ice volume. In the Mt. Harlik region, areal extent was reduced by 10.5% (0.32% a?1), length by 166 m, and volume by 14% between 1972 and 2005. South-facing glaciers lost more of their area than those that are north facing, yielding an areal loss of 25.3% and 16.9% for southern and northern slopes of Mt. Bogda, respectively, and 12.3% and 6.6% for the comparable slopes of Mt. Harlik. Glaciers smaller than 0.5 km2 in area experienced the strongest retreat, whereas glaciers larger than 2 km2 in area experienced gentle recession but may be the main contributors in the future to river runoff. Glacial ablation in eastern Xinjiang tends to be strong, and the water resources in this region are deteriorating. Also, a heavy reduction in the capacity of the local karez system, as well as a significant change in river runoff, can be related to glacial retreat. Combined, this will adversely affect the downstream city of Urumqi and the Turfan Basin.
LI KaiMingLI ZhongQinGAO WenYuWANG Lin
关键词:冰川退缩河川径流吐鲁番盆地卫星图像
天山乌鲁木齐河源区径流水化学特征及影响因素分析被引量:9
2011年
在乌鲁木齐河源区采集两年的大气降水和1号冰川、空冰斗、总控3个水文点逐日定时径流样品,对主要离子、pH、电导率EC和总溶解固体TDS进行了分析。结果表明,大气降水离子类型为Ca2+-Na+-HCO3--SO42-,接近中性;径流离子类型为Ca2+-HCO3--SO42-,呈弱碱性。径流中EC和TDS均值总控>1号冰川>空冰斗,其中1号冰川径流的峰值远高于其它两个水文点。受不同下垫面的影响,1号冰川水文点TDS变化受日径流量影响显著,而空冰斗水文点基本不受影响。径流中离子组成主要受岩石风化作用影响,离子比值和Piper图分析说明控制径流离子的主要过程是碳酸盐、黄铁矿和长石类矿物风化。海盐校正分析得出,大气降水对1号冰川、空冰斗、总控径流离子贡献率分别为4.91%,9.10%和5.42%。通过阳离子通量计算,2006年、2007年1号冰川径流的化学风化侵蚀率分别为18.1t/(km2·a)和12.3t/(km2·a)。
冯芳李忠勤张明军金爽王飞腾
关键词:离子浓度岩石风化
Chemistry and environmental significance of aerosols collected in the eastern Tianshan
2017年
Aerosol samples were collected at altitudes from 584 m a.s.l.to 3,804 m a.s.l.at seven sites of the eastern Tianshan.The occurrence,distribution,and possible sources of 47 trace metals—including alkali metals and alkali earth metals,transition metals,lanthanoids,and heavy metals—were investigated.It was found that four sampling sites(Shuinichang,1,691 m a.s.l.;Urumqi City,809 m a.s.l.;Fu Kang Station,584 m a.s.l.;and Bogeda Glacier No.4,3,613 m a.s.l.)were contaminated mainly by heavy metals.Other three high-altitude sites(Urumqi Glacier No.1,3,804 m a.s.l.;Wang Feng road-maintenance station,3,039 m a.s.l.;and Tianshan Glaciology Station,2,135 m a.s.l.)were not polluted.The aerosol particles were clustered into two dominant types:crust-originated particles and pollution-derived particles.Aerosols from UG1,WF,and TGS were characterized by crust-originated particles such as clay,plagioclase,dolomite,alkali feldspar,and biotite;while those from SNC,Urumqi,FK,and BG4 were characterized by high content of Cl-rich particles,S-rich particles,and soot.The backward-trajectories results indicated that air masses arriving at SNC,Urumqi,FK,and BG4 were identified as the more polluted source,when compared to the short-range air mass transport from the North to UGI and WF.Relatively lower altitude,as well as terrain blocking,might be another important reason for the gradient difference in pollution influence among these seven places in the Urumqi River Basin.
XiaoYu ZhangShengJie WangXin ZhangPing ZhouShuang JinZhongQin LiNozomu Takeuchi
关键词:HEAVY-METALPOLLUTIONAEROSOLSASIA
Heavy Metal-Polluted Aerosols Collected at a Rural Site,Northwest China
2017年
Daily samples of aerosol(n=27) were collected from September 21 st to October 4th, 2013 in Fukang(44.17oN, 88.45oE, 475 m a.s.l.), Xinjiang, Northwest China. The enrichment factors(EFc) of selected 49 elements showed that the aerosols had extremely high concentrations of heavy metals, probably indicating their anthropogenic origins. Morphology of individual aerosol particles was determined by scanning electron microscopy and energy-dispersive X-ray microanalysis. Based on morphology and elemental composition, the particles were clustered into three dominant types:(Ⅰ) crustal originated particles: Si/Al-rich particles(36%) and Si/Fe-rich particles(24%);(Ⅱ) mixed source particles; and(Ⅲ) pollution derived particles: Pb-rich particles(10%). The backward trajectories were calculated using the HYSPLIT model, and the results indicated the different anthropogenic sources for heavy metals in Fukang aerosols. Air mass from north was identified as the most polluted source when compared to south and west.
Xiaoyu ZhangZhongqin LiNozomu TakeuchiFeiteng WangShengjie WangXiaoni YouPing Zhou
关键词:气溶胶粒子
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